Jamie Dimon was in Bournemouth, where he was announcing an investment of about £350m in JP Morgan's campus there, as well as a £3.5m philanthropic investment in local non-profits.
Chancellor Rachel Reeves said the investment was "fantastic news for the local economy and people who live" in Dorset.
Ahead of the interview, Dimon appeared before a town hall on the campus - cutting a figure more akin to an off-duty rock star than a bank CEO - wearing an open-collar shirt and jeans, and high-fiving staff on his way to the stage.
Opening with his take on the UK's economy, Dimon said he felt Rachel Reeves was doing a "terrific job", and he felt optimistic about some of the government's attempts to boost innovation and cut regulation.
However, on the broader economic picture, he felt there were increased risks US stock markets were overheated.
"I am far more worried about that than others," he said.